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Journal articles
Artificial maturation of [FeFe] hydrogenase in a redox polymer film
Christina Felbek
1
Steffen Hardt
2
Cecilia Papini
3
Debajyoti Pramanik
4
Vincent Artero
4
Marc Fontecave
3
Vincent Fourmond
1
Nicolas Plumere
5
Christophe Léger
1
4
SolHyCat - Solar fuels, hydrogen and catalysis
LCBM - UMR 5249 - Laboratoire de Chimie et Biologie des Métaux
Christina Felbek 1
Author
Steffen Hardt 2
Author
Cecilia Papini 3
Author
Debajyoti Pramanik 4
Author
Vincent Artero 4
Author
Marc Fontecave 3
Author
Vincent Fourmond 1
Author IdHAL : vincent-fourmond ORCID : https://orcid.org/0000-0001-9837-6214
Nicolas Plumere 5
Author
Christophe Léger 1
Author IdHAL : christophe-leger ORCID : https://orcid.org/0000-0002-8871-6059 ResearcherId : http://www.researcherid.com/rid/A-4115-2008
1
BIP - Bioénergétique et Ingénierie des Protéines (CNRS - Université d’ Aix-Marseille
31, chemin Joseph Aiguier
13402 MARSEILLE Cedex 20 FRANCE
Tél : +33 (0)4 91 16 45 50 - France)
- AMU - Aix Marseille Université : UMR7281 (Aix-Marseille Université Jardins du Pharo 58 Boulevard Charles Livon 13284 Marseille cedex 7 - France)
- CNRS - Centre National de la Recherche Scientifique : UMR7281 (France)
2
Center of Smart Interfaces (TU Darmstadt, Darmstadt - Germany)
- TU Darmstadt - Technische Universität Darmstadt (Karolinenplatz 5, 64289 Darmstadt - Germany)
3
LCPB - Laboratoire de Chimie des Processus Biologiques (Collège de France 75005 - France)
- CdF (institution) - Collège de France : FRE3488 (France)
- SU - Sorbonne Université (21 rue de l’École de médecine - 75006 Paris - France)
- CNRS - Centre National de la Recherche Scientifique : UMR8229 (France)
4
SolHyCat - Solar fuels, hydrogen and catalysis ( 17, avenue des Martyrs 38 054 Grenoble cedex 09 - France)
- LCBM - UMR 5249 - Laboratoire de Chimie et Biologie des Métaux (17, rue des Martyrs 38054 Grenoble cedex 09 - France)
- CNRS - Centre National de la Recherche Scientifique : UMR5249 (France)
- UGA - Université Grenoble Alpes (Adresse CS 40700 - 38058 Grenoble cedex - France)
- IRIG - Institut de Recherche Interdisciplinaire de Grenoble : DRF/IRIG/DIESE (France)
- DRF (CEA) - Direction de Recherche Fondamentale (CEA) : DRF/IRIG (Direction de Recherche Fondamentale
Fundamental Research Division
CEA Saclay
91191 Gif-sur-Yvette
- France)
- CEA - Commissariat à l'énergie atomique et aux énergies alternatives (Centre de Saclay Centre de Grenoble Centre de Cadarache etc - France)
- DRF (CEA) - Direction de Recherche Fondamentale (CEA) : DRF/IRIG (Direction de Recherche Fondamentale
Fundamental Research Division
CEA Saclay
91191 Gif-sur-Yvette
- France)
5
TUM - Technical University of Munich (Arcisstrasse 21, D- 80333 München - Germany)
Abstract : We demonstrate that the insertion of the dinuclear active site of [FeFe] hydrogenase into the apo-enzyme can occur when the enzyme is embedded in a film of redox polymer, under conditions of mediated electron transfer. The maturation can be monitored by electrochemistry, and is as fast as under conditions of direct electron transfer. This new approach clears further the way to the implementation of hydrogenases in large scale real life processes.
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Journal articles
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https://hal.archives-ouvertes.fr/hal-03102775
Contributor : Aurélia Bimbi <>
Submitted on : Thursday, January 7, 2021 - 5:20:53 PM
Last modification on : Friday, February 19, 2021 - 8:50:02 PM
Contributor : Aurélia Bimbi <>
Submitted on : Thursday, January 7, 2021 - 5:20:53 PM
Last modification on : Friday, February 19, 2021 - 8:50:02 PM
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- HAL Id : hal-03102775, version 1
- DOI : 10.1039/d0cc08168j
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Christina Felbek, Steffen Hardt, Cecilia Papini, Debajyoti Pramanik, Vincent Artero, et al.. Artificial maturation of [FeFe] hydrogenase in a redox polymer film. Chemical Communications, Royal Society of Chemistry, In press, ⟨10.1039/d0cc08168j⟩. ⟨hal-03102775⟩
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